Production of 55Co via the 54Fe(d,n)-process and excitation functions of 54Fe(d,t)53Fe and 54Fe(d,α)52mMn reactions from threshold up to 13.8MeV

Verfasser / Beitragende:
[M. R. Zaman, S. Spellerberg, S.M. Qaim]
Ort, Verlag, Jahr:
2003
Enthalten in:
Radiochimica Acta/International journal for chemical aspects of nuclear science and technology, 91/2/2003(2003-02-01), 105-108
Format:
Artikel (online)
ID: 378877070
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024 7 0 |a 10.1524/ract.91.2.105.19991  |2 doi 
035 |a (NATIONALLICENCE)gruyter-10.1524/ract.91.2.105.19991 
245 0 0 |a Production of 55Co via the 54Fe(d,n)-process and excitation functions of 54Fe(d,t)53Fe and 54Fe(d,α)52mMn reactions from threshold up to 13.8MeV  |h [Elektronische Daten]  |c [M. R. Zaman, S. Spellerberg, S.M. Qaim] 
520 3 |a For production of the medically interesting β+-emitter 55Co (T1/2=17.6h) via the 54Fe(d,n)-reaction, 91.6% enriched 54Fe2O3, mixed with Al powder, was pressed to a pellet which could be irradiated with 14MeV deuterons at 4µA in a water-cooled target system. A separation method was developed which led to >99.9% pure 55Co and allowed a recovery of the enriched target material. For a target thickness of Ed=12.6 → 5MeV, the experimental thick target yield of 55Co after chemical separation amounted to about 13MBq/µA·h, which is about 60% of the theoretical value. In a 3h irradiation at 4µA, the batch yield of 55Co achieved was 160MBq (4.3mCi). An 8h irradiation could lead to a batch yield of about 400MBq. The 54Fe(d,n) reaction leads to the highest purity 55Co but it is essential that the isotopic enrichment of the target is not less than 90%. In addition to the production work, cross sections were measured for the 54Fe(d,t) 53Fe and 54Fe(d,α)52mMn reactions using the standard stacked-foil technique and high-resolution γ-ray spectrometry. The cross section ratio for the isomeric pair 52m,gMn is discussed in terms of the spins of the two states involved and the increasing projectile energy. 
540 |a © 2003 Oldenbourg Wissenschaftsverlag GmbH 
690 7 |a Laboratory techniques, experiments  |2 nationallicence 
690 7 |a Analytical chemistry  |2 nationallicence 
690 7 |a Inorganic chemistry  |2 nationallicence 
700 1 |a Zaman  |D M. R.  |4 aut 
700 1 |a Spellerberg  |D S.  |4 aut 
700 1 |a Qaim  |D S.M.  |4 aut 
773 0 |t Radiochimica Acta/International journal for chemical aspects of nuclear science and technology  |d Oldenbourg Wissenschaftsverlag GmbH  |g 91/2/2003(2003-02-01), 105-108  |x 0033-8230  |q 91:2/2003<105  |1 2003  |2 91  |o ract 
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950 |B NATIONALLICENCE  |P 700  |E 1-  |a Zaman  |D M. R.  |4 aut 
950 |B NATIONALLICENCE  |P 700  |E 1-  |a Spellerberg  |D S.  |4 aut 
950 |B NATIONALLICENCE  |P 700  |E 1-  |a Qaim  |D S.M.  |4 aut 
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