Effect of alpha radiolysis on doped UO2 dissolution under reducing conditions
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| 024 | 7 | 0 | |a 10.1524/ract.92.9.611.55010 |2 doi |
| 035 | |a (NATIONALLICENCE)gruyter-10.1524/ract.92.9.611.55010 | ||
| 245 | 0 | 0 | |a Effect of alpha radiolysis on doped UO2 dissolution under reducing conditions |h [Elektronische Daten] |c [Thierry Mennecart, Bernd Grambow, M. Fattahi, Z. Andriambololona] |
| 520 | 3 | |a The aim of the present work is to quantify the influence of alpha radioactivity of 225Ac doped UO2 on the dissolution rate under reducing conditions at pH 6. The doped or undoped material was prepared by precipitation and the size of particles was about 3nm. The total alpha activity of the doped material was about 2000MBq g-1 UO2, about 4 times higher than that of 15years old spent fuel. The solution was kept under reducing conditions during the experiment by permanent electrochemical reduction under inert atmosphere. The results showed that the dissolution rate of doped material was a function of alpha activity and thus a function of the dose. | |
| 540 | |a © 2004 Oldenbourg Wissenschaftsverlag GmbH | ||
| 690 | 7 | |a Laboratory techniques, experiments |2 nationallicence | |
| 690 | 7 | |a Analytical chemistry |2 nationallicence | |
| 690 | 7 | |a Inorganic chemistry |2 nationallicence | |
| 700 | 1 | |a Mennecart |D Thierry |4 aut | |
| 700 | 1 | |a Grambow |D Bernd |4 aut | |
| 700 | 1 | |a Fattahi |D M. |4 aut | |
| 700 | 1 | |a Andriambololona |D Z. |4 aut | |
| 773 | 0 | |t Radiochimica Acta/International journal for chemical aspects of nuclear science and technology |d Oldenbourg Wissenschaftsverlag GmbH |g 92/9-11/2004(2004-11-01), 611-615 |x 0033-8230 |q 92:9-11/2004<611 |1 2004 |2 92 |o ract | |
| 856 | 4 | 0 | |u https://doi.org/10.1524/ract.92.9.611.55010 |q text/html |z Onlinezugriff via DOI |
| 908 | |D 1 |a research article |2 jats | ||
| 950 | |B NATIONALLICENCE |P 856 |E 40 |u https://doi.org/10.1524/ract.92.9.611.55010 |q text/html |z Onlinezugriff via DOI | ||
| 950 | |B NATIONALLICENCE |P 700 |E 1- |a Mennecart |D Thierry |4 aut | ||
| 950 | |B NATIONALLICENCE |P 700 |E 1- |a Grambow |D Bernd |4 aut | ||
| 950 | |B NATIONALLICENCE |P 700 |E 1- |a Fattahi |D M. |4 aut | ||
| 950 | |B NATIONALLICENCE |P 700 |E 1- |a Andriambololona |D Z. |4 aut | ||
| 950 | |B NATIONALLICENCE |P 773 |E 0- |t Radiochimica Acta/International journal for chemical aspects of nuclear science and technology |d Oldenbourg Wissenschaftsverlag GmbH |g 92/9-11/2004(2004-11-01), 611-615 |x 0033-8230 |q 92:9-11/2004<611 |1 2004 |2 92 |o ract | ||
| 900 | 7 | |b CC0 |u http://creativecommons.org/publicdomain/zero/1.0 |2 nationallicence | |
| 898 | |a BK010053 |b XK010053 |c XK010000 | ||
| 949 | |B NATIONALLICENCE |F NATIONALLICENCE |b NL-gruyter | ||