caa a22 4500 469031867 CHVBK 20180323132745.0 cr unu---uuuuu 170328e19920501xx s 000 0 eng 10.1007/BF01889672 doi (NATIONALLICENCE)springer-10.1007/BF01889672 Klein Lewis Department of Physics and Astronomy, Howard University, 20059, Washington, D.C. aut Line shapes in nonlinear spectroscopy [Elektronische Daten] [Lewis Klein] The shape of the spectral lines of an optically active system interacting with one or more strong radiation fields in the presence of a perturbing bath is studied. A method based on the statistics of the fluctuation of the interaction between the radiator and the perturbing environment (the model Markov microfield theory) is used. This method permits the foundations of line shape theory in modern statistical mechanics to be seen clearly. Multiphoton processes and homogeneous, inhomogeneous, and power broadening mechanisms are included in the analysis. The correlations between radiative and collisional processes which arise in nonlinear spectroscopy are included explicitly. A discussion of the new information that is obtained from these correlations in nonlinear spectroscopy is also presented. Several model systems are presented as illustrative examples of the theory. Plenum Publishing Corporation, 1992 Foundations of Physics Kluwer Academic Publishers-Plenum Publishers 22/5(1992-05-01), 669-690 0015-9018 22:5<669 1992 22 10701 https://doi.org/10.1007/BF01889672 text/html Onlinezugriff via DOI 1 research-article jats NATIONALLICENCE 856 40 https://doi.org/10.1007/BF01889672 text/html Onlinezugriff via DOI NATIONALLICENCE 100 1- Klein Lewis Department of Physics and Astronomy, Howard University, 20059, Washington, D.C aut NATIONALLICENCE 773 0- Foundations of Physics Kluwer Academic Publishers-Plenum Publishers 22/5(1992-05-01), 669-690 0015-9018 22:5<669 1992 22 10701 Metadata rights reserved Springer special CC-BY-NC licence nationallicence BK010053 XK010053 XK010000 NATIONALLICENCE NATIONALLICENCE NL-springer