Measurements and receptor modeling of volatile organic compounds in Southeastern Mexico City, 2000-2007

Verfasser / Beitragende:
[Henry Wöhrnschimmel, Miguel Magaña, Werner A. Stahel, Salvador Blanco, S. Acuña, J.M. Pérez, S. González, V. Gutiérrez, Shinji Wakamatsu, B. Cárdenas]
Ort, Verlag, Jahr:
2010
Enthalten in:
Atmospheric Chemistry and Physics, 10 (18), pp. 9027-9037
Format:
Artikel (online)
ID: 528787152
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024 7 0 |a 10.3929/ethz-b-000027647  |2 doi 
024 7 0 |a 10.5194/acp-10-9027-2010  |2 doi 
035 |a (ETHRESEARCH)oai:www.research-collecti.ethz.ch:20.500.11850/27647 
245 0 0 |a Measurements and receptor modeling of volatile organic compounds in Southeastern Mexico City, 2000-2007  |h [Elektronische Daten]  |c [Henry Wöhrnschimmel, Miguel Magaña, Werner A. Stahel, Salvador Blanco, S. Acuña, J.M. Pérez, S. González, V. Gutiérrez, Shinji Wakamatsu, B. Cárdenas] 
246 0 |a Atmos. chem. phys. 
506 |a Open access  |2 ethresearch 
520 3 |a Ambient samples of volatile organic compounds (VOCs) were measured between 2000 and 2007 in Southeastern Mexico City, quantifying 13 species (ethane, propane, propylene, butane, acetylene, pentane, hexane, heptane, benzene, octane, toluene, nonane, o-xylene). These time series were analyzed for long-term trends, using linear regression models. A main finding was that the concentrations for several VOC species were decreasing during this period. A receptor model was applied to identify possible VOC sources, as well as temporal patterns in their respective contributions. Domestic use of liquefied petroleum gas (LPG) and vehicle exhaust are suggested to be the principal emission sources, contributing together between 70% and 80% to the total of quantified species. Both diurnal and seasonal patterns, as well as a weekend effect were recognized in the modelled source contributions. Furthermore, decreasing trends over time were found for LPG and hot soak (−7.8% and −12.7% per year, respectively, p < 0.01), whereas for vehicle exhaust no significant trend was found. 
540 |a Creative Commons Attribution 3.0 Unported  |u http://creativecommons.org/licenses/by/3.0  |2 ethresearch 
700 1 |a Wöhrnschimmel  |D Henry  |e joint author 
700 1 |a Magaña  |D Miguel  |e joint author 
700 1 |a Stahel  |D Werner A.  |e joint author 
700 1 |a Blanco  |D Salvador  |e joint author 
700 1 |a Acuña  |D S.  |e joint author 
700 1 |a Pérez  |D J.M.  |e joint author 
700 1 |a González  |D S.  |e joint author 
700 1 |a Gutiérrez  |D V.  |e joint author 
700 1 |a Wakamatsu  |D Shinji  |e joint author 
700 1 |a Cárdenas  |D B.  |e joint author 
773 0 |t Atmospheric Chemistry and Physics  |d Munich : European Geophysical Society  |g 10 (18), pp. 9027-9037  |x 1680-7375 
856 4 0 |u http://hdl.handle.net/20.500.11850/27647  |q text/html  |z WWW-Backlink auf das Repository (Open access) 
908 |D 1  |a Journal Article  |2 ethresearch 
950 |B ETHRESEARCH  |P 856  |E 40  |u http://hdl.handle.net/20.500.11850/27647  |q text/html  |z WWW-Backlink auf das Repository (Open access) 
950 |B ETHRESEARCH  |P 700  |E 1-  |a Wöhrnschimmel  |D Henry  |e joint author 
950 |B ETHRESEARCH  |P 700  |E 1-  |a Magaña  |D Miguel  |e joint author 
950 |B ETHRESEARCH  |P 700  |E 1-  |a Stahel  |D Werner A.  |e joint author 
950 |B ETHRESEARCH  |P 700  |E 1-  |a Blanco  |D Salvador  |e joint author 
950 |B ETHRESEARCH  |P 700  |E 1-  |a Acuña  |D S.  |e joint author 
950 |B ETHRESEARCH  |P 700  |E 1-  |a Pérez  |D J.M.  |e joint author 
950 |B ETHRESEARCH  |P 700  |E 1-  |a González  |D S.  |e joint author 
950 |B ETHRESEARCH  |P 700  |E 1-  |a Gutiérrez  |D V.  |e joint author 
950 |B ETHRESEARCH  |P 700  |E 1-  |a Wakamatsu  |D Shinji  |e joint author 
950 |B ETHRESEARCH  |P 700  |E 1-  |a Cárdenas  |D B.  |e joint author 
950 |B ETHRESEARCH  |P 773  |E 0-  |t Atmospheric Chemistry and Physics  |d Munich : European Geophysical Society  |g 10 (18), pp. 9027-9037  |x 1680-7375 
898 |a BK010053  |b XK010053  |c XK010000 
949 |B ETHRESEARCH  |F ETHRESEARCH  |b ETHRESEARCH  |j Journal Article  |c Open access