Quantum dynamics of a plasmonic metamolecule with a time-dependent driving

Verfasser / Beitragende:
[Daniel Uken, Alessandro Sergi]
Ort, Verlag, Jahr:
2015
Enthalten in:
Theoretical Chemistry Accounts, 134/12(2015-12-01), 1-8
Format:
Artikel (online)
ID: 605487537
LEADER caa a22 4500
001 605487537
003 CHVBK
005 20210128100451.0
007 cr unu---uuuuu
008 210128e20151201xx s 000 0 eng
024 7 0 |a 10.1007/s00214-015-1749-9  |2 doi 
035 |a (NATIONALLICENCE)springer-10.1007/s00214-015-1749-9 
245 0 0 |a Quantum dynamics of a plasmonic metamolecule with a time-dependent driving  |h [Elektronische Daten]  |c [Daniel Uken, Alessandro Sergi] 
520 3 |a We simulate the dynamics of a quantum dot coupled to the single resonating mode of a metal nanoparticle. Systems like this are known as metamolecules. In this study, we consider a time-dependent driving field acting onto the metamolecule. We use the Heisenberg equations of motion for the entire system, while representing the resonating mode in Wigner phase space. A time-dependent basis is adopted for the quantum dot. We integrate the dynamics of the metamolecule for a range of coupling strengths between the quantum dot and the driving field, while restricting the coupling between the quantum dot and the resonant mode to weak values. By monitoring the average of the time variation in the energy of the metamolecule model, as well as the coherence and the population difference in the quantum dot, we observe distinct nonlinear behavior in the case of strong coupling to the driving field. 
540 |a Springer-Verlag Berlin Heidelberg, 2015 
690 7 |a Quantum dynamics  |2 nationallicence 
690 7 |a Plasmonic metamolecule  |2 nationallicence 
690 7 |a Time-dependent driving  |2 nationallicence 
700 1 |a Uken  |D Daniel  |u School of Chemistry and Physics, University of KwaZulu-Natal, Private Bag X01, 3209, Scottsville, Pietermaritzburg, South Africa  |4 aut 
700 1 |a Sergi  |D Alessandro  |u School of Chemistry and Physics, University of KwaZulu-Natal, Private Bag X01, 3209, Scottsville, Pietermaritzburg, South Africa  |4 aut 
773 0 |t Theoretical Chemistry Accounts  |d Springer Berlin Heidelberg  |g 134/12(2015-12-01), 1-8  |x 1432-881X  |q 134:12<1  |1 2015  |2 134  |o 214 
856 4 0 |u https://doi.org/10.1007/s00214-015-1749-9  |q text/html  |z Onlinezugriff via DOI 
898 |a BK010053  |b XK010053  |c XK010000 
900 7 |a Metadata rights reserved  |b Springer special CC-BY-NC licence  |2 nationallicence 
908 |D 1  |a research-article  |2 jats 
949 |B NATIONALLICENCE  |F NATIONALLICENCE  |b NL-springer 
950 |B NATIONALLICENCE  |P 856  |E 40  |u https://doi.org/10.1007/s00214-015-1749-9  |q text/html  |z Onlinezugriff via DOI 
950 |B NATIONALLICENCE  |P 700  |E 1-  |a Uken  |D Daniel  |u School of Chemistry and Physics, University of KwaZulu-Natal, Private Bag X01, 3209, Scottsville, Pietermaritzburg, South Africa  |4 aut 
950 |B NATIONALLICENCE  |P 700  |E 1-  |a Sergi  |D Alessandro  |u School of Chemistry and Physics, University of KwaZulu-Natal, Private Bag X01, 3209, Scottsville, Pietermaritzburg, South Africa  |4 aut 
950 |B NATIONALLICENCE  |P 773  |E 0-  |t Theoretical Chemistry Accounts  |d Springer Berlin Heidelberg  |g 134/12(2015-12-01), 1-8  |x 1432-881X  |q 134:12<1  |1 2015  |2 134  |o 214