Quantum dynamics of a plasmonic metamolecule with a time-dependent driving
Gespeichert in:
Verfasser / Beitragende:
[Daniel Uken, Alessandro Sergi]
Ort, Verlag, Jahr:
2015
Enthalten in:
Theoretical Chemistry Accounts, 134/12(2015-12-01), 1-8
Format:
Artikel (online)
Online Zugang:
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| 024 | 7 | 0 | |a 10.1007/s00214-015-1749-9 |2 doi |
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| 245 | 0 | 0 | |a Quantum dynamics of a plasmonic metamolecule with a time-dependent driving |h [Elektronische Daten] |c [Daniel Uken, Alessandro Sergi] |
| 520 | 3 | |a We simulate the dynamics of a quantum dot coupled to the single resonating mode of a metal nanoparticle. Systems like this are known as metamolecules. In this study, we consider a time-dependent driving field acting onto the metamolecule. We use the Heisenberg equations of motion for the entire system, while representing the resonating mode in Wigner phase space. A time-dependent basis is adopted for the quantum dot. We integrate the dynamics of the metamolecule for a range of coupling strengths between the quantum dot and the driving field, while restricting the coupling between the quantum dot and the resonant mode to weak values. By monitoring the average of the time variation in the energy of the metamolecule model, as well as the coherence and the population difference in the quantum dot, we observe distinct nonlinear behavior in the case of strong coupling to the driving field. | |
| 540 | |a Springer-Verlag Berlin Heidelberg, 2015 | ||
| 690 | 7 | |a Quantum dynamics |2 nationallicence | |
| 690 | 7 | |a Plasmonic metamolecule |2 nationallicence | |
| 690 | 7 | |a Time-dependent driving |2 nationallicence | |
| 700 | 1 | |a Uken |D Daniel |u School of Chemistry and Physics, University of KwaZulu-Natal, Private Bag X01, 3209, Scottsville, Pietermaritzburg, South Africa |4 aut | |
| 700 | 1 | |a Sergi |D Alessandro |u School of Chemistry and Physics, University of KwaZulu-Natal, Private Bag X01, 3209, Scottsville, Pietermaritzburg, South Africa |4 aut | |
| 773 | 0 | |t Theoretical Chemistry Accounts |d Springer Berlin Heidelberg |g 134/12(2015-12-01), 1-8 |x 1432-881X |q 134:12<1 |1 2015 |2 134 |o 214 | |
| 856 | 4 | 0 | |u https://doi.org/10.1007/s00214-015-1749-9 |q text/html |z Onlinezugriff via DOI |
| 898 | |a BK010053 |b XK010053 |c XK010000 | ||
| 900 | 7 | |a Metadata rights reserved |b Springer special CC-BY-NC licence |2 nationallicence | |
| 908 | |D 1 |a research-article |2 jats | ||
| 949 | |B NATIONALLICENCE |F NATIONALLICENCE |b NL-springer | ||
| 950 | |B NATIONALLICENCE |P 856 |E 40 |u https://doi.org/10.1007/s00214-015-1749-9 |q text/html |z Onlinezugriff via DOI | ||
| 950 | |B NATIONALLICENCE |P 700 |E 1- |a Uken |D Daniel |u School of Chemistry and Physics, University of KwaZulu-Natal, Private Bag X01, 3209, Scottsville, Pietermaritzburg, South Africa |4 aut | ||
| 950 | |B NATIONALLICENCE |P 700 |E 1- |a Sergi |D Alessandro |u School of Chemistry and Physics, University of KwaZulu-Natal, Private Bag X01, 3209, Scottsville, Pietermaritzburg, South Africa |4 aut | ||
| 950 | |B NATIONALLICENCE |P 773 |E 0- |t Theoretical Chemistry Accounts |d Springer Berlin Heidelberg |g 134/12(2015-12-01), 1-8 |x 1432-881X |q 134:12<1 |1 2015 |2 134 |o 214 | ||