Re-acclimation performance and microbial characteristics of a thermophilic biofilter for NOx removal from flue gas

Verfasser / Beitragende:
[Shihan Zhang, Han Chen, Yinfeng Xia, Jingkai Zhao, Nan Liu, Wei Li]
Ort, Verlag, Jahr:
2015
Enthalten in:
Applied Microbiology and Biotechnology, 99/16(2015-08-01), 6879-6887
Format:
Artikel (online)
ID: 605498466
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024 7 0 |a 10.1007/s00253-015-6585-2  |2 doi 
035 |a (NATIONALLICENCE)springer-10.1007/s00253-015-6585-2 
245 0 0 |a Re-acclimation performance and microbial characteristics of a thermophilic biofilter for NOx removal from flue gas  |h [Elektronische Daten]  |c [Shihan Zhang, Han Chen, Yinfeng Xia, Jingkai Zhao, Nan Liu, Wei Li] 
520 3 |a Currently, a novel chemical absorption-biological reduction (CABR) integrated process, employing Fe(II)EDTA as a solvent, is being under development to reduce the cost of NOx removal from flue gas. In this work, the NO removal profile, re-acclimation performance, and microbial characteristics in a thermophilic biofilter were investigated at the conditions typical to CABR process. The biofilter comprised of four layers of packing material with a surface area of 1200m2m−3. Experimental results revealed that the biofilter could remove 95% of the fed NO at typical flue gas conditions. As the gas residence time varied from 90 to 15s, the NO removal efficiency decreased from 100 to 56.5% due to the NO mass transfer limitation. The longer period of the biofilter shutdown required more time for its re-acclimation. For example, after 8-day shutdown, the biofilter was re-acclimated in 32h. Denaturing gradient gel electrophoresis analysis of PCR-amplified product showed that Pseudomonas, a group of denitrifier, was dominant in the biofilter. Because the Pseudomonas was abundant at the bottom layer of packed-bed, the bottom layer contributed to 60-70% of the total NO removal. In addition, Pseudomonas gradually faded away along the gas flow path from the bottom to the top of biofilter, resulting in a significant decrease in NO removal at the other three packed-bed layers. These observed results will provide the process engineering and scale-up data with respect to the biofilter operations to help advance the CABR process to pilot-scale testing. 
540 |a Springer-Verlag Berlin Heidelberg, 2015 
690 7 |a NOx removal  |2 nationallicence 
690 7 |a CABR  |2 nationallicence 
690 7 |a Re-acclimation  |2 nationallicence 
690 7 |a Flue gas  |2 nationallicence 
690 7 |a Microbial community  |2 nationallicence 
700 1 |a Zhang  |D Shihan  |u Key Laboratory of Biomass Chemical Engineering of Ministry of Education, Institute of Industrial Ecology and Environment, College of Chemical and Biological Engineering, Zhejiang University, Yuquan Campus, 310027, Hangzhou, China  |4 aut 
700 1 |a Chen  |D Han  |u Institute of Environmental Engineering, Zhejiang University, Zijingang Campus, 310058, Hangzhou, China  |4 aut 
700 1 |a Xia  |D Yinfeng  |u Key Laboratory of Biomass Chemical Engineering of Ministry of Education, Institute of Industrial Ecology and Environment, College of Chemical and Biological Engineering, Zhejiang University, Yuquan Campus, 310027, Hangzhou, China  |4 aut 
700 1 |a Zhao  |D Jingkai  |u Key Laboratory of Biomass Chemical Engineering of Ministry of Education, Institute of Industrial Ecology and Environment, College of Chemical and Biological Engineering, Zhejiang University, Yuquan Campus, 310027, Hangzhou, China  |4 aut 
700 1 |a Liu  |D Nan  |u Key Laboratory of Biomass Chemical Engineering of Ministry of Education, Institute of Industrial Ecology and Environment, College of Chemical and Biological Engineering, Zhejiang University, Yuquan Campus, 310027, Hangzhou, China  |4 aut 
700 1 |a Li  |D Wei  |u Key Laboratory of Biomass Chemical Engineering of Ministry of Education, Institute of Industrial Ecology and Environment, College of Chemical and Biological Engineering, Zhejiang University, Yuquan Campus, 310027, Hangzhou, China  |4 aut 
773 0 |t Applied Microbiology and Biotechnology  |d Springer Berlin Heidelberg  |g 99/16(2015-08-01), 6879-6887  |x 0175-7598  |q 99:16<6879  |1 2015  |2 99  |o 253 
856 4 0 |u https://doi.org/10.1007/s00253-015-6585-2  |q text/html  |z Onlinezugriff via DOI 
898 |a BK010053  |b XK010053  |c XK010000 
900 7 |a Metadata rights reserved  |b Springer special CC-BY-NC licence  |2 nationallicence 
908 |D 1  |a research-article  |2 jats 
949 |B NATIONALLICENCE  |F NATIONALLICENCE  |b NL-springer 
950 |B NATIONALLICENCE  |P 856  |E 40  |u https://doi.org/10.1007/s00253-015-6585-2  |q text/html  |z Onlinezugriff via DOI 
950 |B NATIONALLICENCE  |P 700  |E 1-  |a Zhang  |D Shihan  |u Key Laboratory of Biomass Chemical Engineering of Ministry of Education, Institute of Industrial Ecology and Environment, College of Chemical and Biological Engineering, Zhejiang University, Yuquan Campus, 310027, Hangzhou, China  |4 aut 
950 |B NATIONALLICENCE  |P 700  |E 1-  |a Chen  |D Han  |u Institute of Environmental Engineering, Zhejiang University, Zijingang Campus, 310058, Hangzhou, China  |4 aut 
950 |B NATIONALLICENCE  |P 700  |E 1-  |a Xia  |D Yinfeng  |u Key Laboratory of Biomass Chemical Engineering of Ministry of Education, Institute of Industrial Ecology and Environment, College of Chemical and Biological Engineering, Zhejiang University, Yuquan Campus, 310027, Hangzhou, China  |4 aut 
950 |B NATIONALLICENCE  |P 700  |E 1-  |a Zhao  |D Jingkai  |u Key Laboratory of Biomass Chemical Engineering of Ministry of Education, Institute of Industrial Ecology and Environment, College of Chemical and Biological Engineering, Zhejiang University, Yuquan Campus, 310027, Hangzhou, China  |4 aut 
950 |B NATIONALLICENCE  |P 700  |E 1-  |a Liu  |D Nan  |u Key Laboratory of Biomass Chemical Engineering of Ministry of Education, Institute of Industrial Ecology and Environment, College of Chemical and Biological Engineering, Zhejiang University, Yuquan Campus, 310027, Hangzhou, China  |4 aut 
950 |B NATIONALLICENCE  |P 700  |E 1-  |a Li  |D Wei  |u Key Laboratory of Biomass Chemical Engineering of Ministry of Education, Institute of Industrial Ecology and Environment, College of Chemical and Biological Engineering, Zhejiang University, Yuquan Campus, 310027, Hangzhou, China  |4 aut 
950 |B NATIONALLICENCE  |P 773  |E 0-  |t Applied Microbiology and Biotechnology  |d Springer Berlin Heidelberg  |g 99/16(2015-08-01), 6879-6887  |x 0175-7598  |q 99:16<6879  |1 2015  |2 99  |o 253